Update! Brake problem is, in fact, solved! The switch back to the original brake booster solved the self-application problem. Rebuilding the original stop lamp switch solved the taillamp problem. Zip ties and gorilla glue for the win!
As far as the engine goes, everything, and I do mean EVERYTHING on this truck is/was original Chrysler parts. OK- the engine belts were new, and the guy who had it before me had the brake system rebuilt, but everything else was factory parts. To be honest, I think a slant is a smidge too small to power this big heavy brick around, especially since it has four wheel drive. Plus, I would have to track down another slant six transmission case and swap guts to make it 4WD compatible. Not interested and don't have the time right now.
I have my 76 D100 to scratch my slant itch. The Ramcharger is my daily driver, but the 76 D100 is my toy. I have big plans for it and its 225/727 drivetrain, it is just a matter of time and money. If you are familiar with Roadkill and Steve Dulcich's Mopar Muscle Truck, that is kind of what I am going for, just with a slant instead of a v-8. And Little Red Express exhaust stacks.
The Ramcharger's stock 318 will (eventually) be upgraded with a set of factory high-swirl "302" late 80s cylinder heads, an Edelbrock SP2P two barrel intake manifold (WITH EGR provisions), and possible a cam swap to a cam I got from Joshie225 years ago. The axles have 3.2 gears in them so this is never going to be a off-roading or racing vehicle. With 3.2 gears it will rarely get over 3000 RPM, even on the highway, so I am modifying the engine to maximize low-RPM torque. I have all the parts for this, it is, again, a matter of time and money. I want to get the heads checked out and possibly rebuilt before I install them.
I am happy that I can now actually drive this thing safely. But the next project is replacing the badly rusted out original exhaust system. Everything from the head pipe back has rusted out and failed internally. I think the backpressure is so bad that the engine only gets about 15-16 inches of vacuum at idle.
Thank you all for the input and assistance!